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41.
The study of re-homogenized melt inclusions in the same growth planes of quartz of pegmatites genetically linked to the Variscan
granite of the Ehrenfriedersdorf complex, Erzgebirge, Germany, by ion microprobe analyses has determined high concentrations
of Be, up to 10,000 ppm, in one type of melt inclusion, as well as moderate concentrations in the 100 ppm range in a second
type of melt inclusion. Generally, the high Be concentrations are associated with the H2O- and other volatile-rich type-B melt inclusions, and the lower Be concentration levels are connected to H2O-poor type-A melt inclusions. Both inclusion types, representing conjugate melt pairs, are formed by a liquid–liquid immiscibility
separation process. This extremely strong and very systematic scattering in Be provides insights into the origin of Be concentration
and transport mechanisms in pegmatite-forming melts. In this contribution, we present more than 250 new analytical data and
show with ion microprobe and fs-LA-ICPMS studies on quenched glasses, as well as with confocal Raman spectroscopy of daughter
minerals in unheated melt inclusions, that the concentrations of Be may achieve such extreme levels during melt–melt immiscibility
of H2O-, B-, F-, P-, ± Li-enriched pegmatite-forming magmas. Starting from host granite with about 10 ppm Be, melt inclusions with
10,000 ppm Be correspond to enrichment by a factor of over 1,000. This strong enrichment of Be is the result of processes
of fractional crystallization and further enrichment in melt patches of pegmatite bodies due to melt–melt immiscibility at
fluid saturation. We also draw additional conclusions regarding the speciation of Be in pegmatite-forming melt systems from
investigation of the Be-bearing daughter mineral phases in the most H2O-rich melt inclusions. In the case of evolved volatile and H2O-rich pegmatite systems, B, P, and carbonates are important for the enrichment and formation of stable Be complexes. 相似文献
42.
Jan P. Amend Thomas M. McCollom Wolfgang Bach 《Geochimica et cosmochimica acta》2011,75(19):5736-5748
Active deep-sea hydrothermal vents are hosted by a range of different rock types, including basalt, peridotite, and felsic rocks. The associated hydrothermal fluids exhibit substantial chemical variability, which is largely attributable to compositional differences among the underlying host rocks. Numerical models were used to evaluate the energetics of seven inorganic redox reactions (potential catabolisms of chemolithoautotrophs) and numerous biomolecule synthesis reactions (anabolism) in a representative sampling of these systems, where chemical gradients are established by mixing hydrothermal fluid with seawater. The wide ranging fluid compositions dictate demonstrable differences in Gibbs energies (ΔGr) of these catabolic and anabolic reactions in three peridotite-hosted, six basalt-hosted, one troctolite-basalt hybrid, and two felsic rock-hosted systems. In peridotite-hosted systems at low to moderate temperatures (<∼45 °C) and high seawater:hydrothermal fluid (SW:HF) mixing ratios (>10), hydrogen oxidation yields the most catabolic energy, but the oxidation of methane, ferrous iron, and sulfide can also be moderately exergonic. At higher temperatures, and consequent SW:HF mixing ratios <10, anaerobic processes dominate the energy landscape; sulfate reduction and methanogenesis are more exergonic than any of the aerobic respiration reactions. By comparison, in the basalt-hosted and felsic rock-hosted systems, sulfide oxidation was the predominant catabolic energy source at all temperatures (and SW:HF ratios) considered. The energetics of catabolism at the troctolite-basalt hybrid system were intermediate to these extremes. Reaction energetics for anabolism in chemolithoautotrophs—represented here by the synthesis of amino acids, nucleotides, fatty acids, saccharides, and amines—were generally most favorable at moderate temperatures (22-32 °C) and corresponding SW:HF mixing ratios (∼15). In peridotite-hosted and the troctolite-basalt hybrid systems, ΔGr for primary biomass synthesis yielded up to ∼900 J per g dry cell mass. The energetics of anabolism in basalt- and felsic rock-hosted systems were far less favorable. The results suggest that in peridotite-hosted (and troctolite-basalt hybrid) systems, compared with their basalt (and felsic rock) counterparts, microbial catabolic strategies—and consequently variations in microbial phylotypes—may be far more diverse and some biomass synthesis may yield energy rather than imposing a high energetic cost. 相似文献
43.
The Totalp-Platta-Malenco ophiolites in the Eastern Central Alps offer a unique opportunity to study the behaviour of Li, Be and B in ultramafic rocks in response to serpentinization and to progressive Alpine metamorphism. These units represent the remnants of a former ocean-continent transition that was intensely serpentinized during exposure on the Jurassic seafloor of the Ligurian Tethys. From north to the south, three isograd reactions (lizardite⇒antigorite+brucite;lizardite+talc⇒antigorite;lizardite+tremolite⇒antigorite+diopside) have been used to quantify the evolution of the light element content of metamorphic minerals. We determined the Li, Be and B concentrations in major silicate minerals from the ultramafic bodies of Totalp, Platta and Malenco by secondary ion mass spectrometry. Mantle minerals have Be concentrations (e.g. <0.001-0.009 μg/g in olivine) similar to the metamorphic minerals that replace them (e.g. <0.001-0.016 μg/g in serpentine). The mantle signature of Be is thus neither erased during seafloor alteration nor by progressive metamorphism from prehnite-pumpellyite to epidote-amphibolite facies. In contrast, the Li and B inventories of metamorphic minerals are related to the lizardite-to-antigorite transition. Both elements display higher concentrations in the low-temperature serpentine polymorph lizardite (max. 156 μg/g Li, max. 318 μg/g B) than in antigorite (max. 0.11 μg/g Li, max. 12 μg/g B). Calculated average B/Li ratios for lizardite (∼1395) and antigorite (∼115) indicate that Li fractionates from B during the lizardite-to-antigorite transition during prograde metamorphism in ultramafic rocks. In subduction zones, this signature is likely to be recorded in the B-rich nature of forearc fluids.Relative to oceanic mantle the Be content of mantle clinopyroxene is much higher, but similar to Be values from mantle xenoliths and subduction-related peridotite massifs. These data support previous hypothesis that the mantle rocks from the Eastern Central Alps have a subcontinental origin. We conclude that Be behaves conservatively during subduction metamorphism of ultramafic rocks, at least at low-temperature, and thus retains the fingerprint of ancient subduction-related igneous events in mantle peridotites. 相似文献
44.
45.
The leaching behaviour of electrostatic precipitator dust from the Mufulira Cu smelter (Copperbelt, Zambia) was studied using a 48-h pH-static leaching experiment (CEN/TS 14997). The release of metals (Cd, Co, Cu, Ni, Pb and Zn) and changes in mineralogical composition using X-ray diffraction and PHREEQC-2 modelling were investigated in the pH range of 3–7. The highest concentrations of metals were released at pH 3–4.5, which encompasses the natural pH of the dust suspension (~4.3). About 40% of the total Cu was leached at pH 3, yielding 107 g/kg. Chalcanthite (CuSO4·5H2O), magnetite (Fe3O4) and delafossite (CuFeO2) represented the principal phases of the studied dust. In contact with water, chalcanthite was dissolved and hydrated Cu sulphates precipitated at pH 4–7. Gypsum (CaSO4·2H2O) and secondary Fe or Al phases were observed in the leached residues. Serious environmental impact due to leaching may occur in dust-contaminated soil systems in the vicinity of the smelting plants. 相似文献
46.
Laure Moulin Ana Isabel Catarino Thomas Claessens Philippe Dubois 《Marine pollution bulletin》2011,62(1):48-54
The effect of pH ranging from 8.0 to 6.8 (total scale - pHT) on fertilization, cleavage and larval development until pluteus stage was assessed in an intertidal temperate sea urchin. Gametes were obtained from adults collected in two contrasting tide pools, one showing a significant nocturnal pH decrease (lowest pHT = 7.4) and another where pH was more stable (lowest pHT = 7.8). The highest pHT at which significant effects on fertilization and cleavage were recorded was 7.6. On the contrary, larval development was only affected below pHT 7.4, a value equal or lower than that reported for several subtidal species. This suggests that sea urchins inhabiting stressful intertidal environments produce offspring that may better resist future ocean acidification. Moreover, at pHT 7.4, the fertilization rate of gametes whose progenitors came from the tide pool with higher pH decrease was significantly higher, indicating a possible acclimatization or adaptation of gametes to pH stress. 相似文献
47.
Chunming Shi Valérie Masson-Delmotte Camille Risi Thomas Eglin Michel Stievenard Monique Pierre Xiaochun Wang Jing Gao François-Marie Bréon Qi-Bin Zhang Valérie Daux 《Earth and Planetary Science Letters》2011,301(1-2):307-316
We explore the potential of tree-ring cellulose δ18O and δ13C records for reconstructing climate variability in the southeast Tibetan Plateau. Our sampling strategy was designed to investigate intra and inter-tree variability, and the effects of the age of tree on δ18O variation. We show that intra-tree δ13C and δ18O variability is negligible, and inter-tree coherence is sufficient to build robust tree-ring δ18O or δ13C chronologies based on only four trees. There is no evidence of an age effect regarding δ18O, in contrast with tree-ring width. In our warm and moist sampling site, young tree δ13C is not clearly correlated with monthly mean meteorological data. Tree-ring δ18O appears significantly anti-correlated with summer precipitation amount, regional cloud cover, and relative humidity. Simulations conducted with the ORCHIDEE land surface model confirm the observed contribution of relative humidity to tree cellulose δ18O, and explain the weak correlation of δ13C with climate by the non-linear integration linked with photosynthesis. Altogether, the tree-ring cellulose δ18O is shown to be a promising proxy to reconstruct regional summer moisture variability prior to the instrumental period. 相似文献
48.
Phytoplankton dynamics and cyanobacterial dominance in Murchison Bay of Lake Victoria (Uganda) in relation to environmental conditions 总被引:2,自引:0,他引:2
Sigrid Haande Thomas RohrlackRonald P. Semyalo Pål BrettumBente Edvardsen Anne Lyche-SolheimKai Sørensen Petter Larsson 《Limnologica》2011,41(1):20-29
Murchison Bay is a shallow embayment in the north-western part of Lake Victoria, strongly influenced by urban pollution from the Ugandan capital Kampala. Two stations, representing the semi-enclosed innermost part of the bay and the wider outer part of the bay, were sampled in the period from April 2003 to March 2004, in order to assess the phytoplankton community and the nutrient status in the bay. Murchison Bay was highly eutrophic with average concentrations (n=25) of total phosphorous >90 μg L−1 and total nitrogen >1100 μg L−1 in the inner part of the bay. The phytoplankton community was dominated by a variety of cyanobacterial species and diatoms. Cyanobacteria were dominant in the whole bay, whereas diatoms were more abundant in the outer part of the bay. Moreover, the proportion of N-fixing species like Anabaena sp. was higher in the outer part of the bay, whereas species like Microcystis sp. were more abundant in the inner part of the bay. The phytoplankton community, especially in the outer part of the bay, may be influenced by light limitation. Low NO3-N concentrations in the bay may also indicate a possible N-limitation, thus favouring growth of N-fixing cyanobacteria. The open bay is, however, a complex system, and additional environmental factors and loss processes most likely affect the phytoplankton community. 相似文献
49.
Progress in some areas of process‐based aeolian sediment transport research is hampered by limited opportunities for data comparison, synthesis, and integration. This is partially due to a lack of reliable comparison methods. Many comparison methods are forms of calibration that are either restrictive (e.g., time‐averages only) or non‐existent (e.g., for field‐based sediment transport thresholds or vertical mass flux profiles). It is believed that the adoption of standard methods for common measurements may improve inter‐study comparison, add value and longevity to data, and advance integrative modeling efforts. Examples of approaches in allied disciplines where standards are used routinely are reviewed and we discuss how the mutual benefits of standardized data could outweigh perceived disadvantages. Overall, the goal of this commentary is to encourage discussion, self‐assessment, and forethought with regard to measurement methods used in process‐based aeolian geomorphology. Copyright © 2011 John Wiley & Sons, Ltd. 相似文献
50.
Synergy and fusion of optical and synthetic aperture radar satellite data for underwater topography estimation in coastal areas 总被引:1,自引:1,他引:0
Andrey Pleskachevsky Susanne Lehner Thomas Heege Claudius Mott 《Ocean Dynamics》2011,61(12):2099-2120
A method to obtain underwater topography for coastal areas using state-of-the-art remote sensing data and techniques worldwide
is presented. The data from the new Synthetic Aperture Radar (SAR) satellite TerraSAR-X with high resolution up to 1 m are
used to render the ocean waves. As bathymetry is reflected by long swell wave refraction governed by underwater structures
in shallow areas, it can be derived using the dispersion relation from observed swell properties. To complete the bathymetric
maps, optical satellite data of the QuickBird satellite are fused to map extreme shallow waters, e.g., in near-coast areas.
The algorithms for bathymetry estimation from optical and SAR data are combined and integrated in order to cover different
depth domains. Both techniques make use of different physical phenomena and mathematical treatment. The optical methods based
on sunlight reflection analysis provide depths in shallow water up to 20 m in preferably calm weather conditions. The depth
estimation from SAR is based on the observation of long waves and covers the areas between about 70- and 10-m water depths
depending on sea state and acquisition quality. The depths in the range of 20 m up to 10 m represent the domain where the
synergy of data from both sources arises. Thus, the results derived from SAR and optical sensors complement each other. In
this study, a bathymetry map near Rottnest Island, Australia, is derived. QuickBird satellite optical data and radar data
from TerraSAR-X have been used. The depths estimated are aligned on two different grids. The first one is a uniform rectangular
mesh with a horizontal resolution of 150 m, which corresponds to an average swell wavelength observed in the 10 × 10-km SAR
image acquired. The second mesh has a resolution of 150 m for depths up to 20 m (deeper domain covered by SAR-based technique)
and 2.4 m resolution for the shallow domain imaged by an optical sensor. This new technique provides a platform for mapping
of coastal bathymetry over a broad area on a scale that is relevant to marine planners, managers, and offshore industry. 相似文献